Phonons are envisioned as coherent intermediaries between different types of quantum systems. Engineered nanoscale devices, such as optomechanical crystals (OMCs), provide a platform to utilize phonons as quantum information carriers. Here we demonstrate OMCs in diamond designed for strong for interactions between phonons and a silicon vacancy (SiV) spin. Using optical measurements at millikelvin temperatures, we measure a line width of 13 kHz (Q-factor of ∼4.4 × 10⁵) for a 6 GHz acoustic mode, a record for diamond in the GHz frequency range and within an order of magnitude of state-of-the-art line widths for OMCs in silicon. We investigate SiV optical and spin properties in these devices and outline a path toward a coherent spin-phonon interface.

Nuclear spins interact weakly with their environment and therefore exhibit long coherence times. This has led to their use as memory qubits in quantum information platforms, where they are controlled via electromagnetic waves. Scaling up such platforms comes with challenges in terms of power efficiency, as well as cross-talk between devices. Here, we demonstrate coherent control of a single nuclear spin using surface acoustic waves. We use mechanically driven Ramsey and spin-echo sequences to show that the nuclear spin retains its excellent coherence properties. We estimate that this approach requires 2-3 orders of magnitude less power than more conventional control methods. Furthermore, this technique is scalable because of the possibility of guiding acoustic waves and reduced cross-talk between different acoustic channels. This work demonstrates the use of mechanical waves for complex quantum control sequences, offers an advantageous alternative to the standard electromagnetic control of nuclear spins, and opens prospects for incorporating nuclear spins in mechanically interfaced hybrid quantum architectures.

We demonstrate the transmission of a ∼4-GHz surface acoustic wave across a suspended diamond waveguide. This enables simultaneous coherent mechanical driving of, and optical access to, diamond-based color centers.