Emissions of aviation include CO2, H2O, NOx, sulfur oxides, and soot. Many studies have investigated the annual mean climate impact of aviation emissions. While CO2 has a long atmospheric residence time and is almost uniformly distributed in the atmosphere, non-CO2 gases and particles and their products have short atmospheric residence times and are heterogeneously distributed. The climate impact of non-CO2 aviation emissions is known to vary with different meteorological background situations. The aim of this study is to systematically investigate the influence of characteristic weather situations on aviation climate effects over the North Atlantic region, to identify the most sensitive areas, and to potentially detect systematic weather-related similarities. If aircraft were re-routed to avoid climate-sensitive regions, the overall aviation climate impact might be reduced. Hence, the sensitivity of the atmosphere to local emissions provides a basis for the assessment of weather-related, climate-optimized flight trajectory planning. To determine the climate change contribution of an individual emission as a function of location, time, and weather situation, the radiative impact of local emissions of NOx and H2O to changes in O3, CH4, H2O and contrail cirrus was computed by means of the ECHAM5/MESSy Atmospheric Chemistry model. From this, 4-dimensional climate change functions (CCFs) were derived. Typical weather situations in the North Atlantic region were considered for winter and summer. Weather-related differences in O3, CH4, H2O, and contrail cirrus CCFs were investigated. The following characteristics were identified: enhanced climate impact of contrail cirrus was detected for emissions in areas with large-scale lifting, whereas low climate impact of contrail cirrus was found in the area of the jet stream. Northwards of 60° N, contrails usually cause climate warming in winter, independent of the weather situation. NOx emissions cause a high positive climate impact if released in the area of the jet stream or in high-pressure ridges, which induces a south- and downward transport of the emitted species, whereas NOx emissions at, or transported towards, high latitudes cause low or even negative climate impact. Independent of the weather situation, total NOx effects show a minimum at ∼250g hPa, increasing towards higher and lower altitudes, with generally higher positive impact in summer than in winter. H2O emissions induce a high climate impact when released in regions with lower tropopause height, whereas low climate impact occurs for emissions in areas with higher tropopause height. H2O CCFs generally increase with height and are larger in winter than in summer. The CCFs of all individual species can be combined, facilitating the assessment of total climate impact of aircraft trajectories considering CO2 and spatially and temporally varying non-CO2 effects. Furthermore, they allow for the optimization of aircraft trajectories with reduced overall climate impact. This also facilitates a fair evaluation of trade-offs between individual species. In most regions, NOx and contrail cirrus dominate the sensitivity to local aviation emissions. The findings of this study recommend considering weather-related differences for flight trajectory optimization in favour of reducing total climate impact.

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Aviation is seeking for ways to reduce its climate impact caused by CO₂ emissions and non-CO₂ effects. Operational measures which change overall flight altitude have the potential to reduce climate impact of individual effects, comprising CO₂ but in particular non-CO₂ effects. We study the impact of changes of flight altitude, specifically aircraft flying 2000 feet higher and lower, with a set of global models comprising chemistry-transport, chemistry-climate and general circulation models integrating distinct aviation emission inventories representing such alternative flight altitudes, estimating changes in climate impact of aviation by quantifying radiative forcing and induced temperature change. We find in our sensitivity study that flying lower leads to a reduction of radiative forcing of non-CO₂ effects together with slightly increased CO₂ emissions and impacts, when cruise speed is not modified. Flying higher increases radiative forcing of non-CO₂ effects by about 10%, together with a slight decrease of CO₂ emissions and impacts. Overall, flying lower decreases aviation-induced temperature change by about 20%, as a decrease of non-CO₂ impacts by about 30% dominates over slightly increasing CO₂ impacts assuming a sustained emissions scenario. Those estimates are connected with a large but unquantified uncertainty. To improve the understanding of mechanisms controlling the aviation climate impact, we study the geographical distributions of aviation-induced modifications in the atmosphere, together with changes in global radiative forcing and suggest further efforts in order to reduce long standing uncertainties.

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Emissions of aviation include CO2, H2O, NOx and particles. While CO2 has a long atmospheric residence time and is uniformly distributed in the atmosphere, non-CO2 gases, particles and their products have short atmospheric residence times and are heterogeneously distributed. Their climate effects depend on chemical and meteorological background conditions during emission, which vary with geographic location, altitude, time, local insolation, actual weather, etc. This spatial and temporal variability can be utilized for aviation climate impact mitigation by identifying aircraft trajectories which avoid climate-sensitive regions. To determine the climate change contribution of individual emissions as function of 3-dimensional position, time and weather situation, contributions of local emissions to changes in O3, CH4, H2O and contrail-cirrus were computed by means of the ECHAM5/MESSy Atmospheric Chemistry model and four-dimensional climate change functions (CCFs) were derived thereof. Typical weather situations in the North Atlantic region were considered for winter and summer. For all non-CO2 species included in the study, we found distinct weather related differences with respect to their climate impact. Depending on the species, we found enhanced significance of the position of emission release in relation to high pressure systems, in relation to the jet stream, in relation to polar night and in relation to the tropopause altitude. The dominating parameters were found to be contrail-cirrus and total NOx. The results of this study represent a comprehensive basis for weather dependent flight trajectory optimization studies. Furthermore it constitutes the groundwork for the development of more generally applicable algorithmic CCFs. @en