Magnonics is a research field complementary to spintronics, in which the quanta of spin waves (magnons) replace electrons as information carriers, promising lower dissipation^1–3. The development of ultrafast, nanoscale magnonic logic circuits calls for new tools and materials to generate coherent spin waves with frequencies as high and wavelengths as short as possible^4,5. Antiferromagnets can host spin waves at terahertz frequencies and are therefore seen as a future platform for the fastest and least dissipative transfer of information^6–11. However, the generation of short-wavelength coherent propagating magnons in antiferromagnets has so far remained elusive. Here we report the efficient emission and detection of a nanometre-scale wavepacket of coherent propagating magnons in the antiferromagnetic oxide dysprosium orthoferrite using ultrashort pulses of light. The subwavelength confinement of the laser field due to large absorption creates a strongly non-uniform spin excitation profile, enabling the propagation of a broadband continuum of coherent terahertz spin waves. The wavepacket contains magnons with a shortest detected wavelength of 125 nm that propagate into the material with supersonic velocities of more than 13 km s^–1. This source of coherent short-wavelength spin carriers opens up new prospects for terahertz antiferromagnetic magnonics and coherence-mediated logic devices at terahertz frequencies.

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Ultrafast photodoping of the Mott insulators, possessing strong correlation between electronic and magnetic degrees of freedom, holds promise for launching an ultrafast dynamics of spins which cannot be described in terms of conventional models of ultrafast magnetism. Here we study the ultrafast laser-induced dynamics of the magnetic order in a novel spin-orbit Mott insulator Sr2IrO4 featuring an uncompensated pattern of antiferromagnetic spin ordering. Using the transient magneto-optical Kerr effect sensitive to the net magnetization, we reveal that photodoping by femtosecond laser pulses with photon energy above the Mott gap launches melting of the antiferromagnetic order seen as ultrafast demagnetization with a characteristic time of 300 fs followed by a sub-10-ps recovery. Nonequilibrium dynamical mean-field theory calculations based on the single-band Hubbard model confirm that ultrafast demagnetization is primarily governed by the laser-induced generation of electron-hole pairs, although the precise simulated time dependencies are rather different from the experimentally observed ones. To describe the experimental results, here we suggest a phenomenological model which is based on Onsager's formalism and accounts for the photogenerated electron-hole pairs using the concepts of holons and doublons.@en

Excitation of antiferromagnetic HoFeO₃ with a single 80 fs laser pulse triggers a first-order spin-reorientation phase transition. In the ultrafast kinetics of the transition one can distinguish the processes of impulsive excitation of spin precession, nucleation of the new domain and growth of the nuclei. The orientation of the spins in the nuclei is defined by the phase of the laser-induced coherent spin precession. The growth of the nuclei is further promoted by heating induced by the laser excitation. Hereby we demonstrate that in HoFeO₃ coherent control of the spin precession allows an effective control of the route of the heat-induced first-order magnetic phase transition. The theoretical description of the excitation of the spin precession by linearly-polarized ultrashort laser pulses is developed with the sigma model. The analysis showed high sensitivity of the excited dynamics to the initial spin orientations with respect to the crystallographic axes of the material.

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