Modeling the consolidation of fiber-reinforced thermoplastic composites at the part level presents a formidable computational challenge due to the multi-scale nature of the process. In this article, a method to bypass the multi-scale problem by homogenizing the micro scale and describing the medium with characteristic parameters is described. The model is intended for press molding of hybrid textiles and considers a free-form plate with non-uniform thickness and can describe consolidation in three dimensions with some restrictions. 2D implementation in FEM shows how in-plane matrix pressure gradients can arise in parts and cause fiber disorientation. Experimental verification demonstrates that fiber disorientation arises at the predicted location, and that defect size is proportional to matrix pressure gradient. This novel consolidation model provides new insights, enables part and process optimization, and paves the way for high-quality composite part production. Highlights: A consolidation model for press molding of hybrid textiles is presented. A method to extend consolidation models for complex geometry is presented. The origin of defect formation in complex geometries is explained.

The aim of this study was to characterise the microstructural organisation of staple carbon fibre-reinforced polymer composites and to investigate their mechanical properties. Conventionally, fibre-reinforced materials are manufactured using continuous fibres. However, discontinuous fibres are crucial for developing sustainable structural second-life applications. Specifically, aligning staple fibres into yarn or tape-like structures enables similar usage to continuous fibre-based products. Understanding the effects of fibre orientation, fibre length, and compaction on mechanical performance can facilitate the fibres’ use as standard engineering materials. This study employed methods ranging from microscale to macroscale, such as image analysis, X-ray computed tomography, and mechanical testing, to quantify the microstructural organisations resulting from different alignment processing methods. These results were compared with the results of mechanical tests to validate and comprehend the relationship between fibre alignment and strength. The results show a significant influence of alignment on fibre orientation distribution, fibre volume fraction, tortuosity, and mechanical properties. Furthermore, different characteristics of the staple fibre tapes were identified and attributed to kinematic effects during movement of the sliver alignment unit, resulting in varying tape thicknesses and fuzzy surfaces.

A new model is proposed for the consolidation of hybrid textiles, in which air entrapment and dissolution are considered. One of the key parameters is tow permeability, which is described by the analytical model of Gebart and validated at very high fibre volume fractions by direct tow permeability measurement. The model also takes into account the presence of fibres limiting gas diffusion in the molten polymer. Experimental validation of the proposed model is then conducted with quasi-unidirectional glass textile and either polypropylene or polyethylene by measuring the impregnation degree as a function of the consolidation time. Good agreement is found between predictions and measurements for the two matrix systems at different pressures. It is shown that entrapped air significantly influences impregnation. The model offers new and comprehensive insights about the phenomena taking place during consolidation and enables future process optimization.

Thermoplastic compression resin transfer moulding coupled with injection moulding is an appealing process for the production of thermoplastic composites. However, its implementation at an industrial scale remains challenging as variotherm injection moulding could prevent solid skin formation in the parting line, making cavity sealing difficult. In this study, a tool for thermoplastic compression resin transfer moulding and the related methods and process parameters for an implementation at an industrial scale are presented. The validity of the concept is proved by producing and characterizing composite plates with elevated fibre volume fractions and advantageous mechanical properties at a range of production temperatures within a cycle time not exceeding 20 min. The best mechanical properties were obtained at a production temperature of 270°C with a bending strength of 477 MPa, a flexural modulus measured at 25.7 GPa and a fibre volume content of 67%.

This study presents two novel methods for in situ characterization of the reaction-diffusion process during the co-curing of a polyetherimide thermoplastic interlayer with an epoxy-amine thermoset. The first method was based on hot stage experiments using a computer vision point tracker algorithm to detect and trace diffusion fronts, and the second method used space-and time-resolved Raman spectroscopy. Both approaches provided essential information, e.g., type of transport phenomena and diffusion rate. They can also be combined and serve to elucidate phenomena occurring during diffusion up to phase separation of the gradient interphase between the epoxy system and the thermoplastic. Accordingly, it was possible to distinguish reaction-diffusion mechanisms, describe the diffusivity of the present system and evaluate the usability of the above-mentioned methods.