The characteristics of aviation-induced aerosol, its processing, and effects on cirrus clouds and climate are still associated with large uncertainties. Properties of aviation-induced aerosol, however, are crucially needed for the assessment of aviation’s climate impacts today and in the future. We identified more than 1100 aircraft plume encounters during passenger aircraft flights of the IAGOS-CARIBIC Flying Laboratory from July 2018 to March 2020. The aerosol properties inside aircraft plumes were similar, independent of the altitude (i.e., upper troposphere, tropopause region, and lowermost stratosphere). The exhaust aerosol was found to be mostly externally mixed compared to the internally mixed background aerosol, even at a plume age of 1 to 3 h. No enhancement of accumulation mode particles (diameter >250 nm) could be detected inside the aircraft plumes. Particle number emission indices (EIs) deduced from the observations in aged plumes are in the same range as values reported from engine certifications. This finding, together with the observed external mixing state inside the plumes, indicates that the aviation exhaust aerosol almost remains in its emission state during plume expansion. It also reveals that the particle number EIs used in global models are within the range of the EIs measured in aged plumes.

This study places HALO research aircraft observations in the upper-tropospheric Asian summer monsoon anticyclone (ASMA) into the context of regional, intra-annual variability by hindcasts with the ECHAM/MESSy Atmospheric Chemistry (EMAC) model. The observations were obtained during the Earth System Model Validation (ESMVal) campaign in September 2012. Observed and simulated tracer-tracer relations reflect photochemical O3 production as well as in-mixing from the lower troposphere and the tropopause layer. The simulations demonstrate that tropospheric trace gas profiles in the monsoon season are distinct from those in the rest of the year, and the measurements reflect the main processes acting throughout the monsoon season. Net photochemical O3 production is significantly enhanced in the ASMA, where uplifted precursors meet increased NO, mainly produced by lightning. An analysis of multiple monsoon seasons in the simulation shows that stratospherically influenced tropopause layer air is regularly entrained at the eastern ASMA flank and then transported in the southern fringe around the interior region. Radial transport barriers of the circulation are effectively overcome by subseasonal dynamical instabilities of the anticyclone, which occur quite frequently and are of paramount importance for the trace gas composition of the ASMA. Both the isentropic entrainment of O3-rich air and the photochemical conversion of uplifted O3-poor air tend to increase O3 in the ASMA outflow.