This case study explores the evolution of clouds during an Arctic cold air outbreak in the Fram Strait region observed during the HALO-(𝒜𝒞)3 aircraft campaign. Our research provides information about the formation, structure, micro- and macrophysical properties, radiative effects and investigates the role of vertical wind shear and buoyancy forces in the transition from regular cloud streets to rather isotropic cloud patterns. Our findings show that lower horizontal boundary layer wind speeds (< 12 m s-1) disrupt the formation of cloud streets, leading to more isotropic cloud patterns, characterized by increasing cloud fraction (from 0.73 to 0.84), cloud top height (from 330 m to 390 m), and quantify the increase of liquid water path as well. In addition, we observe an increase of the number concentration of ice crystals in a size range between 100 µm and 1000 µm and notable riming processes within organized cloud streets. Concurrent radiation measurements in our case study reveal that isotropic cloud patterns can exhibit either low or high albedo as well as low or high Fnet,TIR, suggesting that these patterns represent different developing stages.@en

Riming is a key precipitation formation process in mixed-phase clouds which efficiently converts cloud liquid to ice water. Here, we present two methods to quantify riming of ice particles from airborne observations with the normalized rime mass, which is the ratio of rime mass to the mass of a size-equivalent spherical graupel particle. We use data obtained during the HALO-(AC)3 aircraft campaign, where two aircraft collected radar and in situ measurements that were closely spatially and temporally collocated over the Fram Strait west of Svalbard in spring 2022. The first method is based on an inverse optimal estimation algorithm for the retrieval of the normalized rime mass from a closure between cloud radar and in situ measurements during these collocated flight segments (combined method). The second method relies on in situ observations only, relating the normalized rime mass to optical particle shape measurements (in situ method). We find good agreement between both methods during collocated flight segments with median normalized rime masses of 0.024 and 0.021 (mean values of 0.035 and 0.033) for the combined and in situ method, respectively. Assuming that particles with a normalized rime mass smaller than 0.01 are unrimed, we obtain average rimed fractions of 88ĝ€¯% and 87ĝ€¯% over all collocated flight segments. Although in situ measurement volumes are in the range of a few cubic centimeters and are therefore much smaller than the radar volume (about 45ĝ€¯m footprint diameter at an altitude of 500ĝ€¯m above ground, with a vertical resolution of 5ĝ€¯m), we assume they are representative of the radar volume. When this assumption is not met due to less homogeneous conditions, discrepancies between the two methods result. We show the performance of the methods in a case study of a collocated segment of cold-air outbreak conditions and compare normalized rime mass results with meteorological and cloud parameters. We find that higher normalized rime masses correlate with streaks of higher radar reflectivity. The methods presented improve our ability to quantify riming from aircraft observations.

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