The Coefficient of Friction (CoF) is an important parameter affecting acceleration and braking behavior of trains, and consequently the inter-train distance and utilization of track. To optimize operation schedules, maximize railway capacity, and realize automatic train operations, reliable measurements of the CoFs experienced by in-service trains are desirable. In this study, a train-borne measurement approach is proposed based on a torque modulation concept. It involves superimposing a small-amplitude sinusoidal signal on the motor torque. Because the wheel-rail friction force acts as variable damping, it causes a phase difference between the angular velocity response of the wheelset and the input modulated torque signal. This phase difference can be used to determine the creep coefficient, i.e., the slope of the creep curve, and then to estimate the CoF in combination with the measured Coefficient of Adhesion (CoA), i.e., the ratio between the wheel-rail friction force and normal load. Simulations of torque modulation with VI-Rail are conducted. Variation of phase difference with the increase of the modulated torque is derived theoretically and compared with numerically obtained results using the VI-Rail multibody dynamics model under different CoF conditions. The good agreement between the results indicates the effectiveness of the proposed measurement concept.@en