We present the initial results of an ongoing survey with the Karl G. Jansky Very Large Array targeting the CO(J = 1-0) transition in a sample of 30 submillimeter-selected, dusty star-forming galaxies (SFGs) at z = 2-5 with existing mid-J CO detections from the Atacama Large Millimeter/submillimeter Array and NOrthern Extended Millimeter Array, of which 17 have been fully observed. We detect CO(1-0) emission in 11 targets, along with three tentative (∼1.5σ-2σ) detections; three galaxies are undetected. Our results yield total molecular gas masses of 6-23 × 10¹⁰ (α _CO/1) M _⊙, with gas mass fractions, f _gas = M _mol/(M _*+M _mol), of 0.1-0.8 and a median depletion time of (140 ± 70) Myr. We find median CO excitation ratios of r ₃₁ = 0.75 ± 0.39 and r ₄₁ = 0.63 ± 0.44, with significant scatter. We find no significant correlation between the excitation ratio and a number of key parameters such as redshift, CO(1-0) line width, or Σ_SFR. We only find a tentative positive correlation between r ₄₁ and the star-forming efficiency, but we are limited by our small sample size. Finally, we compare our results to predictions from the SHARK semi-analytical model, finding a good agreement between the molecular gas masses, depletion times, and gas fractions of our sources and their SHARK counterparts. Our results highlight the heterogeneous nature of the most massive SFGs at high redshift, and the importance of CO(1-0) observations to robustly constrain their total molecular gas content and interstellar medium properties.

Feedback and outflows in galaxies that are associated with a quasar phase are expected to be pivotal in quenching the most massive galaxies. However, observations targeting the molecular outflow phase, which dominates both the mass and momentum and removes the immediate fuel for star formation, are limited in high-z QSO hosts. Massive quiescent galaxies found at z ∼ 4 are predicted to have quenched star formation already by z ∼ 5 and undergone their most intense growth at z > 6. Here, we present two Atacama Large Millimeter/submillimeter Array (ALMA) detections of molecular outflows, traced by blueshifted absorption of the OH 119 μm doublet, from a sample of three z > 6 infrared luminous QSO hosts: J2310+1855 and P183+05. OH 119 μm is also detected in emission from P183+05, and tentatively in the third source: P036+03. Using similar assumptions as for high-z dusty star-forming galaxy outflows, we find that our QSOs drive molecular outflows with comparable mass outflow rates, which are comparably energetic except for J2310+1855's significantly lower outflow energy flux. We do not find evidence, nor require additional input from the central active galactic nucleus (AGN) to drive the molecular outflow in J2310+1855, but we cannot rule out an AGN contribution in P183+05 if a significant AGN contribution to L _FIR is assumed and/or if the outflow covering fraction is high (≥53%), which evidence from the literature suggests is unlikely in these sources. Differences observed in the blueshifted absorption spectral properties may instead be caused by the QSO hosts’ more compact dust continuums, limiting observations to lower altitude and more central regions of the outflow.