We report strong chiral coupling between magnons and photons in microwave waveguides that contain chains of small magnets on special lines. Large magnon accumulations at one edge of the chain emerge when exciting the magnets by a phased antenna array. This mechanism holds the promise of new functionalities in nonlinear and quantum magnonics.

We propose and model a method to excite a large number of coherent magnons with high momentum in optical cavities. This is achieved by two counterpropagating optical modes that are detuned by the frequency of a selected magnon, similar to stimulated Raman scattering. In submillimeter-size yttrium iron garnet spheres, a milliwatt laser input power generates 106-108 coherent magnons. The large magnon population enhances Brillouin light scattering, a probe suitable to access their quantum properties.

We theoretically investigate the collective excitations of multiple (sub)millimeter-sized ferromagnets mediated by waveguide photons. By the position of the magnets in the waveguide, the magnon-photon coupling can be tuned to be chiral, i.e., magnons only couple with photons propagating in one direction, leading to an asymmetric transfer of angular momentum and energy between the magnets. A large enhancement of the magnon number population can be achieved at an edge of a long chain of magnets. The chain also supports standing waves with low radiation efficiency that are inert to the chirality.

Inelastic scattering of photons is a promising technique to manipulate magnons but it suffers from weak intrinsic coupling. We theoretically discuss an idea to increase optomagnonic coupling in optical whispering gallery mode cavities by generalizing a previous analysis to include the exchange interaction. We predict that the optomagnonic coupling constant to surface magnons in yttrium iron garnet (YIG) spheres with radius 300μm can be up to 40 times larger than that to the macrospin Kittel mode. Whereas this enhancement falls short of the requirements for magnon manipulation in pure YIG, nanostructuring and/or materials with larger magneto-optical constants can bridge this gap.

The chirality of magnetostatic Damon-Eshbach (DE) magnons affects the transport of energy and angular momentum at the surface of magnetic films and spheres. We calculate the surface-disorder-limited dephasing and transport lifetimes of surface modes of sufficiently thick high-quality ferromagnetic films such as yttrium iron garnet. Surface magnons are not protected by chirality, but interact strongly with smooth surface roughness. Nevertheless, for long-range disorder, the transport is much less affected by the suppressed backscattering (vertex correction). Moreover, in the presence of roughness, ferromagnetic resonance under a uniform microwave field can generate a considerable number of surface magnons.

Inelastic scattering of light by spin waves generates an energy flow between the light and magnetization fields, a process that can be enhanced and controlled by concentrating the light in magneto-optical resonators. Here, we model the cooling of a sphere made of a magnetic insulator, such as yttrium iron garnet, using a monochromatic laser source. When the magnon lifetimes are much larger than the optical ones, we can treat the latter as a Markovian bath for magnons. The steady-state magnons are canonically distributed with a temperature that is controlled by the light intensity. We predict that such a cooling process can significantly reduce the temperature of the magnetic order within current technology.

We identify experimentally the magnetostatic modes active for Brillouin light scattering in the optical whispering gallery modes of a yttrium iron garnet sphere. Each mode is identified by magnetic-field dispersion of ferromagnetic-resonance spectroscopy and coupling strength to the known field distribution of the microwave drive antenna. Our optical measurements confirm recent predictions that higher-order magnetostatic modes can also generate optical scattering, according to the selection rules derived from the axial symmetry. From this we summarize the selection rules for Brillouin light scattering. We give experimental evidence that the optomagnonic coupling to nonuniform magnons can be higher than that of the uniform Kittel mode.

Brillouin light scattering is an established technique to study magnons, the elementary excitations of a magnet. Its efficiency can be enhanced by cavities that concentrate the light intensity. Here, we theoretically study inelastic scattering of photons by a magnetic sphere that supports optical whispering gallery modes in a plane normal to the magnetization. Magnons with low angular momenta scatter the light in the forward direction with a pronounced asymmetry in the Stokes and the anti-Stokes scattering strength, consistent with earlier studies. Magnons with large angular momenta constitute Damon-Eschbach modes which are shown to inelastically reflect light. The reflection spectrum contains either a Stokes or anti-Stokes peak, depending on the direction of the magnetization, a selection rule that can be explained by the chirality of the Damon-Eshbach magnons. The controllable energy transfer can be used to manage the thermodynamics of the magnet by light.